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Influence of particle size on the ice nucleating ability of mineral dusts (2009)

Abstract
The recently developed Zurich Ice Nucleation Chamber (ZINC) was used to explore ice nucleation of size-selected mineral dust particles at temperatures between −20°C and −55°C. Four different mineral dust species have been tested: montmorillonite, kaolinite, illite and Arizona test dust (ATD). The selected particle diameters are 100 nm, 200 nm, 400 nm and 800 nm. Relative humidities with respect to ice (RH<sub>i</sub>) required to activate 1% of the dust particles as ice nuclei (IN) are reported as a function of temperature. An explicit size dependence of the ice formation efficiency has been observed for all dust types. 800 nm particles required the lowest RH<sub>i</sub> to activate. Deposition nucleation below water saturation was found only below −30°C or −35°C dependent on particle size. Minimum RH<sub>i</sub> for 1% activation were 105% for illite, kaolinite and montmorillonite at −40°C, respectively 110% for ATD at −45°C. In addition, a possible parameterisation for the measured activation spectra is proposed, which could be used in modeling studies.

Publication details
Download http://www.atmos-chem-phys.net/9/6705/2009/acp-9-6705-2009.pdf
http://www.doaj.org/doaj?func=openurl&genre=article&issn=16807316&date=2009&volume=9&issue=18&spage=6705
Publisher Copernicus GmbH
Repository DOAJ-Articles (Sweden)
Language eng